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An other option is to start hitchhiking (to Frankfurt) at the 'Esso' (Mecumstraße 45, 40225 Düsseldorf) that's close to the public transport station 'Auf'm Hennekamp'. A lot of people stop there, before they go directly to '''Frankfurt am Main Airport'''. This spot is not so far away from the city centre, so you could walk there from the centre (takes about 40 minutes to walk there from Heinrich Heine Allee, by tram you need only 7 minutes).